对于“Visual Studio Team Test”，似乎您将ExpectedException属性应用到测试的方法。

文档中的示例:使用Visual Studio团队测试的单元测试演练

[TestMethod]
[ExpectedException(typeof(ArgumentException),
    "A userId of null was inappropriately allowed.")]
public void NullUserIdInConstructor()
{
   LogonInfo logonInfo = new LogonInfo(null, "P@ss0word");
}

作为一种替代方法，您可以尝试测试异常实际上是在您的测试中的下两行中抛出的。

var testDelegate = () => MyService.Method(params);
Assert.Throws<Exception>(testDelegate);

这是测试方法的一个属性…你不使用Assert。看起来是这样的:

[ExpectedException(typeof(ExceptionType))]
public void YourMethod_should_throw_exception()

Even though this is an old question, I would like to add a new thought to the discussion. I have extended the Arrange, Act, Assert pattern to be Expected, Arrange, Act, Assert. You can make an expected exception pointer, then assert it was assigned to. This feels cleaner than doing your Asserts in a catch block, leaving your Act section mostly just for the one line of code to call the method under test. You also don't have to Assert.Fail(); or return from multiple points in the code. Any other exception thrown will cause the test to fail, because it won't be caught, and if an exception of your expected type is thrown, but the it wasn't the one you were expecting, Asserting against the message or other properties of the exception help make sure your test won't pass inadvertently.

[TestMethod]
public void Bar_InvalidDependency_ThrowsInvalidOperationException()
{
    // Expectations
    InvalidOperationException expectedException = null;
    string expectedExceptionMessage = "Bar did something invalid.";

    // Arrange
    IDependency dependency = DependencyMocks.Create();
    Foo foo = new Foo(dependency);

    // Act
    try
    {
        foo.Bar();
    }
    catch (InvalidOperationException ex)
    {
        expectedException = ex;
    }

    // Assert
    Assert.IsNotNull(expectedException);
    Assert.AreEqual(expectedExceptionMessage, expectedException.Message);
}

我知道这个帖子很老了，有很多很好的答案，但值得一提的是，局部函数可以以一种非常简单的方式提供帮助。

//Arrange

//Act
void LocalFunction() => mr.ActualMethod(params);

//Assert
Assert.Throws<Exception>(LocalFunction);

FluentAssertions例子

为那些使用该库的用户添加一个使用FluentAssertions的示例。

// act
Action result = () => {
    sut.DoSomething();
};

// assert
result.Should().Throw<Exception>();

异步的例子

// act
Func<Task> result = async () => {
    await sut.DoSomethingAsync();
};

// assert
await result.Should().ThrowAsync<Exception>();