修改(现在它接受任何非空字符串和任何正chunkSize) Konstantin Spirin的解决方案:

public static IEnumerable<String> Split(String value, int chunkSize) {
  if (null == value)
    throw new ArgumentNullException("value");
  else if (chunkSize <= 0)
    throw new ArgumentOutOfRangeException("chunkSize", "Chunk size should be positive");

  return Enumerable
    .Range(0, value.Length / chunkSize + ((value.Length % chunkSize) == 0 ? 0 : 1))
    .Select(index => (index + 1) * chunkSize < value.Length 
      ? value.Substring(index * chunkSize, chunkSize)
      : value.Substring(index * chunkSize));
}

测试:

  String source = @"ABCDEF";

  // "ABCD,EF"
  String test1 = String.Join(",", Split(source, 4));
  // "AB,CD,EF"
  String test2 = String.Join(",", Split(source, 2));
  // "ABCDEF"
  String test3 = String.Join(",", Split(source, 123));

for (int i = 0; i <= Convert.ToInt32(Math.Truncate(Convert.ToDecimal(_string.Length / _chunkSize))); i++)
{
    var _currentChunk = _string.Substring(i * _chunkSize, Math.Min(_chunkSize, _string.Length - i * _chunkSize));
    //do something with current chunk 
}

最近我不得不在工作中写一些东西来完成这个任务，所以我想我会把我对这个问题的解决方案贴出来。作为一个额外的好处，这个解决方案的功能提供了一种方法，以相反的方向分割字符串，并且它正确地处理上面Marvin Pinto提到的unicode字符。所以，就是这样:

using System;
using Extensions;

namespace TestCSharp
{
    class Program
    {
        static void Main(string[] args)
        {    
            string asciiStr = "This is a string.";
            string unicodeStr = "これは文字列です。";

            string[] array1 = asciiStr.Split(4);
            string[] array2 = asciiStr.Split(-4);

            string[] array3 = asciiStr.Split(7);
            string[] array4 = asciiStr.Split(-7);

            string[] array5 = unicodeStr.Split(5);
            string[] array6 = unicodeStr.Split(-5);
        }
    }
}

namespace Extensions
{
    public static class StringExtensions
    {
        /// <summary>Returns a string array that contains the substrings in this string that are seperated a given fixed length.</summary>
        /// <param name="s">This string object.</param>
        /// <param name="length">Size of each substring.
        ///     <para>CASE: length &gt; 0 , RESULT: String is split from left to right.</para>
        ///     <para>CASE: length == 0 , RESULT: String is returned as the only entry in the array.</para>
        ///     <para>CASE: length &lt; 0 , RESULT: String is split from right to left.</para>
        /// </param>
        /// <returns>String array that has been split into substrings of equal length.</returns>
        /// <example>
        ///     <code>
        ///         string s = "1234567890";
        ///         string[] a = s.Split(4); // a == { "1234", "5678", "90" }
        ///     </code>
        /// </example>            
        public static string[] Split(this string s, int length)
        {
            System.Globalization.StringInfo str = new System.Globalization.StringInfo(s);

            int lengthAbs = Math.Abs(length);

            if (str == null || str.LengthInTextElements == 0 || lengthAbs == 0 || str.LengthInTextElements <= lengthAbs)
                return new string[] { str.ToString() };

            string[] array = new string[(str.LengthInTextElements % lengthAbs == 0 ? str.LengthInTextElements / lengthAbs: (str.LengthInTextElements / lengthAbs) + 1)];

            if (length > 0)
                for (int iStr = 0, iArray = 0; iStr < str.LengthInTextElements && iArray < array.Length; iStr += lengthAbs, iArray++)
                    array[iArray] = str.SubstringByTextElements(iStr, (str.LengthInTextElements - iStr < lengthAbs ? str.LengthInTextElements - iStr : lengthAbs));
            else // if (length < 0)
                for (int iStr = str.LengthInTextElements - 1, iArray = array.Length - 1; iStr >= 0 && iArray >= 0; iStr -= lengthAbs, iArray--)
                    array[iArray] = str.SubstringByTextElements((iStr - lengthAbs < 0 ? 0 : iStr - lengthAbs + 1), (iStr - lengthAbs < 0 ? iStr + 1 : lengthAbs));

            return array;
        }
    }
}

此外，这里还有一个运行此代码结果的图像链接:http://i.imgur.com/16Iih.png

简单而简短:

// this means match a space or not a space (anything) up to 4 characters
var lines = Regex.Matches(str, @"[\s\S]{0,4}").Cast<Match>().Select(x => x.Value);

我在João的解决方案基础上做了一些改进。 我所做的不同之处在于，在我的方法中，你实际上可以指定是否要返回带有剩余字符的数组，或者如果结束字符不匹配所需的块长度，你是否要截断它们，我认为这是相当灵活的，代码相当直接:

using System;
using System.Linq;
using System.Text.RegularExpressions;

namespace SplitFunction
{
    class Program
    {
        static void Main(string[] args)
        {
            string text = "hello, how are you doing today?";
            string[] chunks = SplitIntoChunks(text, 3,false);
            if (chunks != null)
            {
                chunks.ToList().ForEach(e => Console.WriteLine(e));
            }

            Console.ReadKey();
        }

        private static string[] SplitIntoChunks(string text, int chunkSize, bool truncateRemaining)
        {
            string chunk = chunkSize.ToString(); 
            string pattern = truncateRemaining ? ".{" + chunk + "}" : ".{1," + chunk + "}";

            string[] chunks = null;
            if (chunkSize > 0 && !String.IsNullOrEmpty(text))
                chunks = (from Match m in Regex.Matches(text,pattern)select m.Value).ToArray(); 

            return chunks;
        }     
    }
}

为什么不是循环?这里有一些东西可以很好地做到这一点:

        string str = "111122223333444455";
        int chunkSize = 4;
        int stringLength = str.Length;
        for (int i = 0; i < stringLength ; i += chunkSize)
        {
            if (i + chunkSize > stringLength) chunkSize = stringLength  - i;
            Console.WriteLine(str.Substring(i, chunkSize));

        }
        Console.ReadLine();

我不知道你会如何处理字符串不是因子4的情况，但不是说你的想法是不可能的，只是想知道它的动机，如果一个简单的for循环做得很好?显然，上面的内容可以被清除，甚至可以作为扩展方法加入。

或者正如评论中提到的，你知道它是/4

str = "1111222233334444";
for (int i = 0; i < stringLength; i += chunkSize) 
  {Console.WriteLine(str.Substring(i, chunkSize));}