简单而简短:

// this means match a space or not a space (anything) up to 4 characters
var lines = Regex.Matches(str, @"[\s\S]{0,4}").Cast<Match>().Select(x => x.Value);

如有必要分割几个不同的长度: 例如，日期和时间的指定格式为stringstrangeStr = "07092016090532";07092016090532(日期:07.09.2016时间:09:05:32)

public static IEnumerable<string> SplitBy(this string str, int[] chunkLength)
    {
        if (String.IsNullOrEmpty(str)) throw new ArgumentException();
        int i = 0;
        for (int j = 0; j < chunkLength.Length; j++)
        {
            if (chunkLength[j] < 1) throw new ArgumentException();
            if (chunkLength[j] + i > str.Length)
            {
                chunkLength[j] = str.Length - i;
            }
            yield return str.Substring(i, chunkLength[j]);
            i += chunkLength[j];
        }
    }

使用:

string[] dt = strangeStr.SplitBy(new int[] { 2, 2, 4, 2, 2, 2, 2 }).ToArray();

static IEnumerable<string> Split(string str, double chunkSize)
{
    return Enumerable.Range(0, (int) Math.Ceiling(str.Length/chunkSize))
       .Select(i => new string(str
           .Skip(i * (int)chunkSize)
           .Take((int)chunkSize)
           .ToArray()));
}

另一种方法是:

using System;
using System.Collections.Generic;
using System.Linq;

public class Program
{
    public static void Main()
    {

        var x = "Hello World";
        foreach(var i in x.ChunkString(2)) Console.WriteLine(i);
    }
}

public static class Ext{
    public static IEnumerable<string> ChunkString(this string val, int chunkSize){
        return val.Select((x,i) => new {Index = i, Value = x})
                  .GroupBy(x => x.Index/chunkSize, x => x.Value)
                  .Select(x => string.Join("",x));
    }
}

为什么不是循环?这里有一些东西可以很好地做到这一点:

        string str = "111122223333444455";
        int chunkSize = 4;
        int stringLength = str.Length;
        for (int i = 0; i < stringLength ; i += chunkSize)
        {
            if (i + chunkSize > stringLength) chunkSize = stringLength  - i;
            Console.WriteLine(str.Substring(i, chunkSize));

        }
        Console.ReadLine();

我不知道你会如何处理字符串不是因子4的情况，但不是说你的想法是不可能的，只是想知道它的动机，如果一个简单的for循环做得很好?显然，上面的内容可以被清除，甚至可以作为扩展方法加入。

或者正如评论中提到的，你知道它是/4

str = "1111222233334444";
for (int i = 0; i < stringLength; i += chunkSize) 
  {Console.WriteLine(str.Substring(i, chunkSize));} 

六年后o_O

仅仅因为

    public static IEnumerable<string> Split(this string str, int chunkSize, bool remainingInFront)
    {
        var count = (int) Math.Ceiling(str.Length/(double) chunkSize);
        Func<int, int> start = index => remainingInFront ? str.Length - (count - index)*chunkSize : index*chunkSize;
        Func<int, int> end = index => Math.Min(str.Length - Math.Max(start(index), 0), Math.Min(start(index) + chunkSize - Math.Max(start(index), 0), chunkSize));
        return Enumerable.Range(0, count).Select(i => str.Substring(Math.Max(start(i), 0),end(i)));
    }

or

    private static Func<bool, int, int, int, int, int> start = (remainingInFront, length, count, index, size) =>
        remainingInFront ? length - (count - index) * size : index * size;

    private static Func<bool, int, int, int, int, int, int> end = (remainingInFront, length, count, index, size, start) =>
        Math.Min(length - Math.Max(start, 0), Math.Min(start + size - Math.Max(start, 0), size));

    public static IEnumerable<string> Split(this string str, int chunkSize, bool remainingInFront)
    {
        var count = (int)Math.Ceiling(str.Length / (double)chunkSize);
        return Enumerable.Range(0, count).Select(i => str.Substring(
            Math.Max(start(remainingInFront, str.Length, count, i, chunkSize), 0),
            end(remainingInFront, str.Length, count, i, chunkSize, start(remainingInFront, str.Length, count, i, chunkSize))
        ));
    }

AFAIK所有的边缘情况都处理好了。

Console.WriteLine(string.Join(" ", "abc".Split(2, false))); // ab c
Console.WriteLine(string.Join(" ", "abc".Split(2, true))); // a bc
Console.WriteLine(string.Join(" ", "a".Split(2, true))); // a
Console.WriteLine(string.Join(" ", "a".Split(2, false))); // a

        public static List<string> DevideByStringLength(string text, int chunkSize)
    {
        double a = (double)text.Length / chunkSize;
        var numberOfChunks = Math.Ceiling(a);

        Console.WriteLine($"{text.Length} | {numberOfChunks}");

        List<string> chunkList = new List<string>();
        for (int i = 0; i < numberOfChunks; i++)
        {
            string subString = string.Empty;
            if (i == (numberOfChunks - 1))
            {
                subString = text.Substring(chunkSize * i, text.Length - chunkSize * i);
                chunkList.Add(subString);
                continue;
            }
            subString = text.Substring(chunkSize * i, chunkSize);
            chunkList.Add(subString);
        }
        return chunkList;
    }