试试这个:

    public static string[] Split(string str, int chunkSize)
    {
        return Enumerable.Range(0, str.Length / chunkSize)
            .Select(i => str.Substring(i * chunkSize, chunkSize)).ToArray();
    }

为什么不是循环?这里有一些东西可以很好地做到这一点:

        string str = "111122223333444455";
        int chunkSize = 4;
        int stringLength = str.Length;
        for (int i = 0; i < stringLength ; i += chunkSize)
        {
            if (i + chunkSize > stringLength) chunkSize = stringLength  - i;
            Console.WriteLine(str.Substring(i, chunkSize));

        }
        Console.ReadLine();

我不知道你会如何处理字符串不是因子4的情况，但不是说你的想法是不可能的，只是想知道它的动机，如果一个简单的for循环做得很好?显然，上面的内容可以被清除，甚至可以作为扩展方法加入。

或者正如评论中提到的，你知道它是/4

str = "1111222233334444";
for (int i = 0; i < stringLength; i += chunkSize) 
  {Console.WriteLine(str.Substring(i, chunkSize));} 

修改(现在它接受任何非空字符串和任何正chunkSize) Konstantin Spirin的解决方案:

public static IEnumerable<String> Split(String value, int chunkSize) {
  if (null == value)
    throw new ArgumentNullException("value");
  else if (chunkSize <= 0)
    throw new ArgumentOutOfRangeException("chunkSize", "Chunk size should be positive");

  return Enumerable
    .Range(0, value.Length / chunkSize + ((value.Length % chunkSize) == 0 ? 0 : 1))
    .Select(index => (index + 1) * chunkSize < value.Length 
      ? value.Substring(index * chunkSize, chunkSize)
      : value.Substring(index * chunkSize));
}

测试:

  String source = @"ABCDEF";

  // "ABCD,EF"
  String test1 = String.Join(",", Split(source, 4));
  // "AB,CD,EF"
  String test2 = String.Join(",", Split(source, 2));
  // "ABCDEF"
  String test3 = String.Join(",", Split(source, 123));

简单而简短:

// this means match a space or not a space (anything) up to 4 characters
var lines = Regex.Matches(str, @"[\s\S]{0,4}").Cast<Match>().Select(x => x.Value);

六年后o_O

仅仅因为

    public static IEnumerable<string> Split(this string str, int chunkSize, bool remainingInFront)
    {
        var count = (int) Math.Ceiling(str.Length/(double) chunkSize);
        Func<int, int> start = index => remainingInFront ? str.Length - (count - index)*chunkSize : index*chunkSize;
        Func<int, int> end = index => Math.Min(str.Length - Math.Max(start(index), 0), Math.Min(start(index) + chunkSize - Math.Max(start(index), 0), chunkSize));
        return Enumerable.Range(0, count).Select(i => str.Substring(Math.Max(start(i), 0),end(i)));
    }

or

    private static Func<bool, int, int, int, int, int> start = (remainingInFront, length, count, index, size) =>
        remainingInFront ? length - (count - index) * size : index * size;

    private static Func<bool, int, int, int, int, int, int> end = (remainingInFront, length, count, index, size, start) =>
        Math.Min(length - Math.Max(start, 0), Math.Min(start + size - Math.Max(start, 0), size));

    public static IEnumerable<string> Split(this string str, int chunkSize, bool remainingInFront)
    {
        var count = (int)Math.Ceiling(str.Length / (double)chunkSize);
        return Enumerable.Range(0, count).Select(i => str.Substring(
            Math.Max(start(remainingInFront, str.Length, count, i, chunkSize), 0),
            end(remainingInFront, str.Length, count, i, chunkSize, start(remainingInFront, str.Length, count, i, chunkSize))
        ));
    }

AFAIK所有的边缘情况都处理好了。

Console.WriteLine(string.Join(" ", "abc".Split(2, false))); // ab c
Console.WriteLine(string.Join(" ", "abc".Split(2, true))); // a bc
Console.WriteLine(string.Join(" ", "a".Split(2, true))); // a
Console.WriteLine(string.Join(" ", "a".Split(2, false))); // a

static IEnumerable<string> Split(string str, int chunkSize)
{
    return Enumerable.Range(0, str.Length / chunkSize)
        .Select(i => str.Substring(i * chunkSize, chunkSize));
}

请注意，可能需要额外的代码来优雅地处理边缘情况(null或空输入字符串，chunkSize == 0，输入字符串长度不能被chunkSize整除，等等)。最初的问题没有为这些边缘情况指定任何需求，在现实生活中，需求可能会有所不同，因此它们超出了这个答案的范围。